Pyrochars and hydrochars differently alter the sorption of the herbicide isoproturon in an agricultural soil.
Identifieur interne : 001B71 ( Main/Exploration ); précédent : 001B70; suivant : 001B72Pyrochars and hydrochars differently alter the sorption of the herbicide isoproturon in an agricultural soil.
Auteurs : Nina Eibisch [Allemagne] ; Reiner Schroll [Allemagne] ; Roland Fu [Allemagne] ; Robert Mikutta [Allemagne] ; Mirjam Helfrich [Allemagne] ; Heinz Flessa [Allemagne]Source :
- Chemosphere [ 1879-1298 ] ; 2015.
Descripteurs français
- KwdFr :
- Adsorption (MeSH), Analyse de variance (MeSH), Biodisponibilité (MeSH), Charbon de bois (composition chimique), Herbicides (composition chimique), Modèles chimiques (MeSH), Phénylurées (pharmacocinétique), Polluants du sol (composition chimique), Résidus de pesticides (analyse), Sol (composition chimique), Spectroscopie infrarouge à transformée de Fourier (MeSH), Séquestration du carbone (MeSH).
- MESH :
- analyse : Résidus de pesticides.
- composition chimique : Charbon de bois, Herbicides, Polluants du sol, Sol.
- pharmacocinétique : Phénylurées.
- Adsorption, Analyse de variance, Biodisponibilité, Modèles chimiques, Spectroscopie infrarouge à transformée de Fourier, Séquestration du carbone.
English descriptors
- KwdEn :
- Adsorption (MeSH), Analysis of Variance (MeSH), Biological Availability (MeSH), Carbon Sequestration (MeSH), Charcoal (chemistry), Herbicides (chemistry), Models, Chemical (MeSH), Pesticide Residues (analysis), Phenylurea Compounds (pharmacokinetics), Soil (chemistry), Soil Pollutants (chemistry), Spectroscopy, Fourier Transform Infrared (MeSH).
- MESH :
- chemical , analysis : Pesticide Residues.
- chemical , chemistry : Charcoal, Herbicides, Soil, Soil Pollutants.
- chemical , pharmacokinetics : Phenylurea Compounds.
- Adsorption, Analysis of Variance, Biological Availability, Carbon Sequestration, Models, Chemical, Spectroscopy, Fourier Transform Infrared.
Abstract
Carbonaceous material from pyrolysis (pyrochars) and hydrothermal carbonization (hydrochars) are applied to soil to improve soil fertility and carbon sequestration. As a positive side effect, the mobility of pesticides and the risk of groundwater contamination can be minimized. However, the impact of various raw materials on the sorption capacity of different pyrochars and hydrochars is poorly understood. Thus, sorption experiments were performed with (14)C-labeled isoproturon (IPU, 0.75 kg ha(-1)) in a loamy sand soil amended with either pyrochar or hydrochar (0.5% and 5% dry weight, respectively). Carbonaceous materials were produced from three different raw materials: corn digestate, miscanthus, woodchips of willow and poplar. After 72 h of incubation, a sequential extraction procedure was conducted to quantify in situ IPU bioavailability, total amount of extractable IPU, and non-extractable pesticide residues (NER). Added char amount, carbonization type, and raw materials had statistically significant effects on the sorption of IPU. The amount of in situ available IPU was reduced by a factor of 10-2283 in treatments with pyrochar and by a factor of 3-13 in hydrochar treatments. The surface area of the charred material was the most predictive variable of IPU sorption to char amended soil. Some physical and chemical char properties tend to correlate with pore water-, methanol- or non-extractable IPU amounts. Due to a low micro-porosity and ash content, high water extractable carbon contents and O-functional groups of hydrochars, the proportion of NER in hydrochar amended soils was considerably lower than in soil amended with pyrochars.
DOI: 10.1016/j.chemosphere.2014.05.059
PubMed: 24974225
Affiliations:
Links toward previous steps (curation, corpus...)
Le document en format XML
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Electronic address: schroll@helmholtz-muenchen.de.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Helmholtz Zentrum München, German Research Center for Environmental Health (GmbH), Institute of Soil Ecology, 85764 Neuherberg</wicri:regionArea><wicri:noRegion>85764 Neuherberg</wicri:noRegion><wicri:noRegion>85764 Neuherberg</wicri:noRegion><wicri:noRegion>85764 Neuherberg</wicri:noRegion></affiliation></author><author><name sortKey="Fu, Roland" sort="Fu, Roland" uniqKey="Fu R" first="Roland" last="Fu">Roland Fu</name><affiliation wicri:level="1"><nlm:affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig</wicri:regionArea><wicri:noRegion>38116 Braunschweig</wicri:noRegion><wicri:noRegion>38116 Braunschweig</wicri:noRegion><wicri:noRegion>38116 Braunschweig</wicri:noRegion></affiliation></author><author><name sortKey="Mikutta, Robert" sort="Mikutta, Robert" uniqKey="Mikutta R" first="Robert" last="Mikutta">Robert Mikutta</name><affiliation wicri:level="3"><nlm:affiliation>Leibniz Universität Hannover, Institute of Soil Science, 30419 Hannover, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Leibniz Universität Hannover, Institute of Soil Science, 30419 Hannover</wicri:regionArea><placeName><region type="land" nuts="2">Basse-Saxe</region><settlement type="city">Hanovre</settlement></placeName></affiliation></author><author><name sortKey="Helfrich, Mirjam" sort="Helfrich, Mirjam" uniqKey="Helfrich M" first="Mirjam" last="Helfrich">Mirjam Helfrich</name><affiliation wicri:level="1"><nlm:affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig</wicri:regionArea><wicri:noRegion>38116 Braunschweig</wicri:noRegion><wicri:noRegion>38116 Braunschweig</wicri:noRegion><wicri:noRegion>38116 Braunschweig</wicri:noRegion></affiliation></author><author><name sortKey="Flessa, Heinz" sort="Flessa, Heinz" uniqKey="Flessa H" first="Heinz" last="Flessa">Heinz Flessa</name><affiliation wicri:level="1"><nlm:affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig</wicri:regionArea><wicri:noRegion>38116 Braunschweig</wicri:noRegion><wicri:noRegion>38116 Braunschweig</wicri:noRegion><wicri:noRegion>38116 Braunschweig</wicri:noRegion></affiliation></author></analytic><series><title level="j">Chemosphere</title><idno type="eISSN">1879-1298</idno><imprint><date when="2015" type="published">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Adsorption (MeSH)</term><term>Analysis of Variance (MeSH)</term><term>Biological Availability (MeSH)</term><term>Carbon Sequestration (MeSH)</term><term>Charcoal (chemistry)</term><term>Herbicides (chemistry)</term><term>Models, Chemical (MeSH)</term><term>Pesticide Residues (analysis)</term><term>Phenylurea Compounds (pharmacokinetics)</term><term>Soil (chemistry)</term><term>Soil Pollutants (chemistry)</term><term>Spectroscopy, Fourier Transform Infrared (MeSH)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Adsorption (MeSH)</term><term>Analyse de variance (MeSH)</term><term>Biodisponibilité (MeSH)</term><term>Charbon de bois (composition chimique)</term><term>Herbicides (composition chimique)</term><term>Modèles chimiques (MeSH)</term><term>Phénylurées (pharmacocinétique)</term><term>Polluants du sol (composition chimique)</term><term>Résidus de pesticides (analyse)</term><term>Sol (composition chimique)</term><term>Spectroscopie infrarouge à transformée de Fourier (MeSH)</term><term>Séquestration du carbone (MeSH)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="analysis" xml:lang="en"><term>Pesticide Residues</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Charcoal</term><term>Herbicides</term><term>Soil</term><term>Soil Pollutants</term></keywords><keywords scheme="MESH" type="chemical" qualifier="pharmacokinetics" xml:lang="en"><term>Phenylurea Compounds</term></keywords><keywords scheme="MESH" qualifier="analyse" xml:lang="fr"><term>Résidus de pesticides</term></keywords><keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Charbon de bois</term><term>Herbicides</term><term>Polluants du sol</term><term>Sol</term></keywords><keywords scheme="MESH" qualifier="pharmacocinétique" xml:lang="fr"><term>Phénylurées</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Adsorption</term><term>Analysis of Variance</term><term>Biological Availability</term><term>Carbon Sequestration</term><term>Models, Chemical</term><term>Spectroscopy, Fourier Transform Infrared</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Adsorption</term><term>Analyse de variance</term><term>Biodisponibilité</term><term>Modèles chimiques</term><term>Spectroscopie infrarouge à transformée de Fourier</term><term>Séquestration du carbone</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Carbonaceous material from pyrolysis (pyrochars) and hydrothermal carbonization (hydrochars) are applied to soil to improve soil fertility and carbon sequestration. As a positive side effect, the mobility of pesticides and the risk of groundwater contamination can be minimized. However, the impact of various raw materials on the sorption capacity of different pyrochars and hydrochars is poorly understood. Thus, sorption experiments were performed with (14)C-labeled isoproturon (IPU, 0.75 kg ha(-1)) in a loamy sand soil amended with either pyrochar or hydrochar (0.5% and 5% dry weight, respectively). Carbonaceous materials were produced from three different raw materials: corn digestate, miscanthus, woodchips of willow and poplar. After 72 h of incubation, a sequential extraction procedure was conducted to quantify in situ IPU bioavailability, total amount of extractable IPU, and non-extractable pesticide residues (NER). Added char amount, carbonization type, and raw materials had statistically significant effects on the sorption of IPU. The amount of in situ available IPU was reduced by a factor of 10-2283 in treatments with pyrochar and by a factor of 3-13 in hydrochar treatments. The surface area of the charred material was the most predictive variable of IPU sorption to char amended soil. Some physical and chemical char properties tend to correlate with pore water-, methanol- or non-extractable IPU amounts. Due to a low micro-porosity and ash content, high water extractable carbon contents and O-functional groups of hydrochars, the proportion of NER in hydrochar amended soils was considerably lower than in soil amended with pyrochars.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Curated" Owner="NLM"><PMID Version="1">24974225</PMID><DateCompleted><Year>2015</Year><Month>09</Month><Day>11</Day></DateCompleted><DateRevised><Year>2018</Year><Month>12</Month><Day>02</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1879-1298</ISSN><JournalIssue CitedMedium="Internet"><Volume>119</Volume><PubDate><Year>2015</Year><Month>Jan</Month></PubDate></JournalIssue><Title>Chemosphere</Title><ISOAbbreviation>Chemosphere</ISOAbbreviation></Journal><ArticleTitle>Pyrochars and hydrochars differently alter the sorption of the herbicide isoproturon in an agricultural soil.</ArticleTitle><Pagination><MedlinePgn>155-162</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0045-6535(14)00705-X</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.chemosphere.2014.05.059</ELocationID><Abstract><AbstractText>Carbonaceous material from pyrolysis (pyrochars) and hydrothermal carbonization (hydrochars) are applied to soil to improve soil fertility and carbon sequestration. As a positive side effect, the mobility of pesticides and the risk of groundwater contamination can be minimized. However, the impact of various raw materials on the sorption capacity of different pyrochars and hydrochars is poorly understood. Thus, sorption experiments were performed with (14)C-labeled isoproturon (IPU, 0.75 kg ha(-1)) in a loamy sand soil amended with either pyrochar or hydrochar (0.5% and 5% dry weight, respectively). Carbonaceous materials were produced from three different raw materials: corn digestate, miscanthus, woodchips of willow and poplar. After 72 h of incubation, a sequential extraction procedure was conducted to quantify in situ IPU bioavailability, total amount of extractable IPU, and non-extractable pesticide residues (NER). Added char amount, carbonization type, and raw materials had statistically significant effects on the sorption of IPU. The amount of in situ available IPU was reduced by a factor of 10-2283 in treatments with pyrochar and by a factor of 3-13 in hydrochar treatments. The surface area of the charred material was the most predictive variable of IPU sorption to char amended soil. Some physical and chemical char properties tend to correlate with pore water-, methanol- or non-extractable IPU amounts. Due to a low micro-porosity and ash content, high water extractable carbon contents and O-functional groups of hydrochars, the proportion of NER in hydrochar amended soils was considerably lower than in soil amended with pyrochars.</AbstractText><CopyrightInformation>Copyright © 2014 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Eibisch</LastName><ForeName>Nina</ForeName><Initials>N</Initials><AffiliationInfo><Affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany; Helmholtz Zentrum München, German Research Center for Environmental Health (GmbH), Institute of Soil Ecology, 85764 Neuherberg, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Schroll</LastName><ForeName>Reiner</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Helmholtz Zentrum München, German Research Center for Environmental Health (GmbH), Institute of Soil Ecology, 85764 Neuherberg, Germany. Electronic address: schroll@helmholtz-muenchen.de.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Fuß</LastName><ForeName>Roland</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Mikutta</LastName><ForeName>Robert</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Leibniz Universität Hannover, Institute of Soil Science, 30419 Hannover, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Helfrich</LastName><ForeName>Mirjam</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Flessa</LastName><ForeName>Heinz</ForeName><Initials>H</Initials><AffiliationInfo><Affiliation>Thünen Institute of Climate-Smart Agriculture, 38116 Braunschweig, Germany.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D003160">Comparative Study</PublicationType><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2014</Year><Month>06</Month><Day>27</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Chemosphere</MedlineTA><NlmUniqueID>0320657</NlmUniqueID><ISSNLinking>0045-6535</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D006540">Herbicides</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D010573">Pesticide Residues</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D010671">Phenylurea Compounds</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D012987">Soil</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D012989">Soil Pollutants</NameOfSubstance></Chemical><Chemical><RegistryNumber>16291-96-6</RegistryNumber><NameOfSubstance UI="D002606">Charcoal</NameOfSubstance></Chemical><Chemical><RegistryNumber>66066K098P</RegistryNumber><NameOfSubstance UI="C028904">isoproturon</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000327" MajorTopicYN="N">Adsorption</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D000704" MajorTopicYN="N">Analysis of Variance</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D001682" MajorTopicYN="N">Biological Availability</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D057965" MajorTopicYN="N">Carbon Sequestration</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002606" MajorTopicYN="N">Charcoal</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D006540" MajorTopicYN="N">Herbicides</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D008956" MajorTopicYN="N">Models, Chemical</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D010573" MajorTopicYN="N">Pesticide Residues</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="N">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D010671" MajorTopicYN="N">Phenylurea Compounds</DescriptorName><QualifierName UI="Q000493" MajorTopicYN="N">pharmacokinetics</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D012987" MajorTopicYN="N">Soil</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D012989" MajorTopicYN="N">Soil Pollutants</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D017550" MajorTopicYN="N">Spectroscopy, Fourier Transform Infrared</DescriptorName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Adsorption</Keyword><Keyword MajorTopicYN="N">Bioavailability</Keyword><Keyword MajorTopicYN="N">Biochar</Keyword><Keyword MajorTopicYN="N">Hydrothermal carbonization</Keyword><Keyword MajorTopicYN="N">Pesticide</Keyword><Keyword MajorTopicYN="N">Pyrolysis</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2013</Year><Month>11</Month><Day>10</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2014</Year><Month>05</Month><Day>14</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2014</Year><Month>05</Month><Day>23</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2014</Year><Month>6</Month><Day>30</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2014</Year><Month>6</Month><Day>30</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2015</Year><Month>9</Month><Day>12</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">24974225</ArticleId><ArticleId IdType="pii">S0045-6535(14)00705-X</ArticleId><ArticleId IdType="doi">10.1016/j.chemosphere.2014.05.059</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Allemagne</li></country><region><li>Basse-Saxe</li></region><settlement><li>Hanovre</li></settlement></list><tree><country name="Allemagne"><noRegion><name sortKey="Eibisch, Nina" sort="Eibisch, Nina" uniqKey="Eibisch N" first="Nina" last="Eibisch">Nina Eibisch</name></noRegion><name sortKey="Flessa, Heinz" sort="Flessa, Heinz" uniqKey="Flessa H" first="Heinz" last="Flessa">Heinz Flessa</name><name sortKey="Fu, Roland" sort="Fu, Roland" uniqKey="Fu R" first="Roland" last="Fu">Roland Fu</name><name sortKey="Helfrich, Mirjam" sort="Helfrich, Mirjam" uniqKey="Helfrich M" first="Mirjam" last="Helfrich">Mirjam Helfrich</name><name sortKey="Mikutta, Robert" sort="Mikutta, Robert" uniqKey="Mikutta R" first="Robert" last="Mikutta">Robert Mikutta</name><name sortKey="Schroll, Reiner" sort="Schroll, Reiner" uniqKey="Schroll R" first="Reiner" last="Schroll">Reiner Schroll</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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|texte= Pyrochars and hydrochars differently alter the sorption of the herbicide isoproturon in an agricultural soil.
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| HfdSelect -Kh $EXPLOR_AREA/Data/Main/Exploration/biblio.hfd \
| NlmPubMed2Wicri -a PoplarV1
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